具有一维接触电极的双层硒化铌异质结器件制备及电学特性研究

Fabrication and electrical properties of bilayer NbSe2 based van der Waals heterostructure with one-dimensional electrical contact

  • 摘要: 层状硒化铌晶体因其独特的电子结构和物理特性一直是科技界的研究热点,但少层硒化铌晶体薄片在空气中不稳定、器件性能退化严重等因素制约了对其深入研究。本文提出一种具有一维接触电极的双层硒化铌异质结的制备方法,在惰性环境中对硒化铌进行机械剥离、转移和封装,用标准微纳加工工艺制备了以石墨烯为一维接触电极、薄层六角氮化硼为封装材料的双层硒化铌异质结器件。结果表明:双层硒化铌器件的超导转变温度约为6.8 K,电荷密度波相变温度保持在32 K;超导临界电流密度为30 mA/μm2,超导临界磁场为3 T,性能与硒化铌晶体体材料接近;该器件在空气中电学性能非常稳定,保存数月未出现性能退化。

     

    Abstract: Two-dimensional NbSe2 material has attracted significant interest for unique electronic structure and physical properties. However,few-layer NbSe2 crystal is always chemically unstable in air, which severely degrades the perform ance of devices.Here we report a remedial approach based on eleavage,transfer,alignment and encapsulation of air-sensitive two-dimensional crystals,all inside a controlled inert atmosphere.We prepared bilayer NbSe2 devices passivated with h-BN few-layer by using the standard micro-nano processing technology,with graphene as one-dimensional electrical contact.The resuhs show that the device exhibits robust superconductivities with transition temperature about 6.8 K and charge-density-wave phase change happens in ~32 K. Its critical current density of superconductivity is approximately 30 mA/μm2 at 2 K and critical magnetic field is beyond 3 T at 2 K.In addition,device performance of hetero-structure does not obviously degrade after storage in air for several months.

     

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